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ABSTRACT We present the measured gas-phase metal column densities in 155 sub-damped Ly α systems (subDLAs) with the aim to investigate the contribution of subDLAs to the chemical evolution of the Universe. The sample was identified within the absorber-blind XQ-100 quasar spectroscopic survey over the redshift range 2.4 ≤ zabs ≤ 4.3. Using all available column densities of the ionic species investigated (mainly C iv, Si ii, Mg ii, Si iv, Al ii, Fe ii, C ii, and O i; in order of decreasing detection frequency), we estimate the ionization-corrected gas-phase metallicity of each system using Markov chain Monte Carlo techniques to explore a large grid of cloudy ionization models. Without accounting for ionization and dust depletion effects, we find that the H i-weighted gas-phase metallicity evolution of subDLAs is consistent with damped Ly α systems (DLAs). When ionization corrections are included, subDLAs are systematically more metal poor than DLAs (between ≈0.5σ and ≈3σ significance) by up to ≈1.0 dex over the redshift range 3 ≤ zabs ≤ 4.3. The correlation of gas phase [Si/Fe] with metallicity in subDLAs appears to be consistent with that of DLAs, suggesting that the two classes of absorbers have a similar relative dust depletion pattern. As previously seen for Lyman limit systems, the gas phase [C/O] in subDLAs remains constantly solar for all metallicities indicating that both subDLAs and Lyman limit systems could trace carbon-rich ejecta, potentially in circumgalactic environments. 

Abstract Sub-damped Lyman α systems (subDLAs; H i column densities of 19.0 ≤ logN(H i) < 20.3) are rarely included in the cosmic H i census performed at redshifts zabs ≳ 1.5, yet are expected to contribute significantly to the overall H i mass budget of the Universe. In this paper, we present a blindly selected sample of 155 subDLAs found along 100 quasar sightlines (with a redshift path-length ΔX = 475) in the XQ-100 legacy survey to investigate the contribution of subDLAs to the H i mass density of the Universe. The impact of X-Shooter’s spectral resolution on Ly α absorber identification is evaluated, and found to be sufficient for reliably finding absorbers down to a column density of logN(H i) ≥ 18.9. We compared the implications of searching for subDLAs solely using H i absorption versus the use of metal lines to confirm the identification, and found that metal-selection techniques would have missed 75 subDLAs. Using a bootstrap Monte Carlo simulation, we computed the column density distribution function (f(N, X)) and the cosmological H i mass density ($\Omega _{\rm H\,{\small I}}$) of subDLAs and compared with our previous work based on the XQ-100 damped Lyman α systems. We do not find any significant redshift evolution in f(N, X) or $\Omega _{\rm H\,{\small I}}$ for subDLAs. However, subDLAs contribute 10–20 per cent of the total $\Omega _{\rm H\,{\small I}}$ measured at redshifts 2 < z < 5, and thus have a small but significant contribution to the H i budget of the Universe.